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Steric Effects in the Chemisorption of Vibrationally Excited Methane on Nickel
Buch
Buch
Fachbuch
2016

Steric Effects in the Chemisorption of Vibrationally Excited Methane on Nickel

ISBN
EAN
978-3-662-52161-8
9783662521618
Artikel-Nr.
84VZQ5K
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Kostenloser Versand
Rabatt
-21.6
%
CHF 135.00
CHF
105.83
Anzahl
1
Maximale
Lieferzeit
33
Arbeitstage
Mittwoch
28.09.2022
speech-bubble-svg Beschreibung
Bruce Yoder’s thesis outlines his investigation of the dissociative chemisorption of methane (CH4) on a nickel single crystal. In this work Bruce uses a molecular beam and infrared laser techniques to prepare methane in excited rovibrational states. The excited methane molecules are aligned relative to the target nickel surface. Bruce describes the discovery and exploration of a previously unknown steric effect in the dissociation reaction between a vibrationally excited methane molecule and a nickel crystal. From these studies we see that methane molecules are up to twice as reactive when the vibration is aligned parallel rather than perpendicular to the surface. This discovery will help guide the development of detailed predictive models of methane chemisorption, which in turn may lead to better catalysts for the synthesis of several industrially relevant chemicals, including hydrogen fuel from natural gas.
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Stichwörter
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Research
Inhaltsverzeichnis
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Introduction.- Experimental Setup.- State specific preparation and alignment of gas-phase reagents.- State-resolved steric effects in methane chemisorption on Ni(100).- State-resolved steric effects in CH4(v3) dissociation on Ni(110).- Summary and Outlook.
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Autor/-in
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Publikation
Deutschland
23.08.2016
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Sprache
Englisch
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Buch (Softcover)
175 Seiten
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Unterkategorie
Physikalische Chemie
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